|Publication type:||Article in scientific journal|
|Type of review:||Peer review (publication)|
|Title:||Dynamic percolation theory for particle diffusion in a polymer network|
|Published in:||The Journal of Chemical Physics|
|Publisher / Ed. Institution:||American Institute of Physics|
|Subjects:||Soft condensed matter|
|Subject (DDC):||540: Chemistry|
|Abstract:||Tracer-diffusion of small molecules through dense systems of chain polymers is studied within an athermal lattice model, where hard-core interactions are taken into account by means of the site exclusion principle. An approximate mapping of this problem onto dynamic percolation theory is proposed. This method is shown to yield quantitative results for the tracer correlation factor of the molecules as a function of density and chain length provided the non-Poisson character of temporal renewals in the disorder configurations is properly taken into account.|
|Fulltext version:||Published version|
|License (according to publishing contract):||Licence according to publishing contract|
|Departement:||School of Engineering|
|Organisational Unit:||Institute of Data Analysis and Process Design (IDP)|
|Appears in collections:||Publikationen School of Engineering|
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