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Please use this identifier to cite or link to this item: https://doi.org/10.21256/zhaw-1564
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dc.contributor.authorDelmelle, Renaud-
dc.contributor.authorDuarte, Renata Bessa-
dc.contributor.authorFranken, Tanja-
dc.contributor.authorBurnat, Dariusz Artur-
dc.contributor.authorHolzer, Lorenz-
dc.contributor.authorBorgschulte, Andreas-
dc.contributor.authorHeel, Andre-
dc.date.accessioned2018-01-18T10:48:02Z-
dc.date.available2018-01-18T10:48:02Z-
dc.date.issued2016-
dc.identifier.issn0360-3199de_CH
dc.identifier.urihttps://digitalcollection.zhaw.ch/handle/11475/2117-
dc.description.abstractSorption enhanced CO2 methanation is a complex process in which the key challenge lies in the combined optimization of the catalyst activity and water adsorption properties of the zeolite support. In the present work, improved nickel-based catalysts with an enhanced water uptake capacity were designed and catalytically investigated. Two different zeolite frameworks were considered as supports for nanostructured Ni, and studied with defined operation parameters. 5Ni/13X shows significantly increased, nearly three-fold higher, operation time in the sorption enhanced CO2 methanation mode compared to the reference 5Ni/5A, likely due to its higher water sorption capacity. Both catalysts yield comparable CO2 conversion in conventional CO2 methanation (without water uptake). Regeneration of the catalysts performance is possible via a drying step between methanation cycles under both reducing and oxidizing atmospheres; however, operation time of 5Ni/13X increases further after drying under air.de_CH
dc.language.isoende_CH
dc.publisherElsevierde_CH
dc.relation.ispartofInternational Journal of Hydrogen Energyde_CH
dc.rightsLicence according to publishing contractde_CH
dc.subjectSorption enhancedde_CH
dc.subjectCO2 methanationde_CH
dc.subjectMapde_CH
dc.subjectPower to gasde_CH
dc.subject.ddc540: Chemiede_CH
dc.titleDevelopment of improved nickel catalysts for sorption enhanced CO2 methanationde_CH
dc.typeBeitrag in wissenschaftlicher Zeitschriftde_CH
dcterms.typeTextde_CH
zhaw.departementSchool of Engineeringde_CH
zhaw.organisationalunitInstitute of Computational Physics (ICP)de_CH
zhaw.organisationalunitInstitute of Materials and Process Engineering (IMPE)de_CH
dc.identifier.doi10.21256/zhaw-1564-
dc.identifier.doi10.1016/j.ijhydene.2016.09.045de_CH
zhaw.funding.euNode_CH
zhaw.issue44de_CH
zhaw.originated.zhawYesde_CH
zhaw.pages.end20191de_CH
zhaw.pages.start20185de_CH
zhaw.publication.statuspublishedVersionde_CH
zhaw.volume41de_CH
zhaw.publication.reviewPeer review (Publikation)de_CH
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Delmelle, R., Duarte, R. B., Franken, T., Burnat, D. A., Holzer, L., Borgschulte, A., & Heel, A. (2016). Development of improved nickel catalysts for sorption enhanced CO2 methanation. International Journal of Hydrogen Energy, 41(44), 20185–20191. https://doi.org/10.21256/zhaw-1564
Delmelle, R. et al. (2016) ‘Development of improved nickel catalysts for sorption enhanced CO2 methanation’, International Journal of Hydrogen Energy, 41(44), pp. 20185–20191. Available at: https://doi.org/10.21256/zhaw-1564.
R. Delmelle et al., “Development of improved nickel catalysts for sorption enhanced CO2 methanation,” International Journal of Hydrogen Energy, vol. 41, no. 44, pp. 20185–20191, 2016, doi: 10.21256/zhaw-1564.
DELMELLE, Renaud, Renata Bessa DUARTE, Tanja FRANKEN, Dariusz Artur BURNAT, Lorenz HOLZER, Andreas BORGSCHULTE und Andre HEEL, 2016. Development of improved nickel catalysts for sorption enhanced CO2 methanation. International Journal of Hydrogen Energy. 2016. Bd. 41, Nr. 44, S. 20185–20191. DOI 10.21256/zhaw-1564
Delmelle, Renaud, Renata Bessa Duarte, Tanja Franken, Dariusz Artur Burnat, Lorenz Holzer, Andreas Borgschulte, and Andre Heel. 2016. “Development of Improved Nickel Catalysts for Sorption Enhanced CO2 Methanation.” International Journal of Hydrogen Energy 41 (44): 20185–91. https://doi.org/10.21256/zhaw-1564.
Delmelle, Renaud, et al. “Development of Improved Nickel Catalysts for Sorption Enhanced CO2 Methanation.” International Journal of Hydrogen Energy, vol. 41, no. 44, 2016, pp. 20185–91, https://doi.org/10.21256/zhaw-1564.


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