Please use this identifier to cite or link to this item: https://doi.org/10.21256/zhaw-22582
Publication type: Article in scientific journal
Type of review: Peer review (publication)
Title: Ultra‐broadband and high‐dynamic‐range THz time‐domain spectroscopy system based on organic crystal emitter and detector in transmission and reflection geometry
Authors: Puc, Uros
Bach, Tobias
Günter, Peter
Zgonik, Marko
Jazbinsek, Mojca
et. al: No
DOI: 10.1002/adpr.202000098
10.21256/zhaw-22582
Published in: Advanced Photonics Research
Volume(Issue): 2
Issue: 4
Page(s): 2000098
Issue Date: 2021
Publisher / Ed. Institution: Wiley
ISSN: 2699-9293
Language: English
Subjects: THz photonics; Terahertz; Spectroscopy; Organic crystal; DSTMS; DAST; Transmission; Reflection
Subject (DDC): 621.3: Electrical, communications, control engineering
Abstract: The terahertz range of the electromagnetic spectrum reveals important insights when studying material properties. An ultra-broadband terahertz time-domain spectroscopy system based on state-of-the-art, high-stability organic nonlinear optical crystals used as both THz wave generator and detector is presented. In transmission geometry, a broad spectrum exceeding 20 THz and a high dynamic range of more than 80 dB is achieved using a compact 100 MHz femtosecond laser working at telecom wavelength 1560 nm. In the normal-incidence reflection geometry, a similar bandwidth with a dynamic range surpassing 60 dB is reported. The experimental results are supported by a complete theoretical model, which includes the pump pulse duration, THz phonon/vibrational modes of the organic crystals and optical/THz beam path optimizations. The effectiveness of the newly developed system is demonstrated by measuring pharmaceutical samples with distinct THz features in the ultra-broadband THz range and by measuring narrow water vapor lines at a spectral resolution of 2.7 GHz (0.090 cm−1), resulting in an excellent accuracy with a frequency deviation of less than 0.05% from the reference values.
URI: https://digitalcollection.zhaw.ch/handle/11475/22582
Fulltext version: Published version
License (according to publishing contract): CC BY 4.0: Attribution 4.0 International
Departement: School of Engineering
Organisational Unit: Institute of Computational Physics (ICP)
Appears in collections:Publikationen School of Engineering

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Puc, U., Bach, T., Günter, P., Zgonik, M., & Jazbinsek, M. (2021). Ultra‐broadband and high‐dynamic‐range THz time‐domain spectroscopy system based on organic crystal emitter and detector in transmission and reflection geometry. Advanced Photonics Research, 2(4), 2000098. https://doi.org/10.1002/adpr.202000098
Puc, U. et al. (2021) ‘Ultra‐broadband and high‐dynamic‐range THz time‐domain spectroscopy system based on organic crystal emitter and detector in transmission and reflection geometry’, Advanced Photonics Research, 2(4), p. 2000098. Available at: https://doi.org/10.1002/adpr.202000098.
U. Puc, T. Bach, P. Günter, M. Zgonik, and M. Jazbinsek, “Ultra‐broadband and high‐dynamic‐range THz time‐domain spectroscopy system based on organic crystal emitter and detector in transmission and reflection geometry,” Advanced Photonics Research, vol. 2, no. 4, p. 2000098, 2021, doi: 10.1002/adpr.202000098.
PUC, Uros, Tobias BACH, Peter GÜNTER, Marko ZGONIK und Mojca JAZBINSEK, 2021. Ultra‐broadband and high‐dynamic‐range THz time‐domain spectroscopy system based on organic crystal emitter and detector in transmission and reflection geometry. Advanced Photonics Research. 2021. Bd. 2, Nr. 4, S. 2000098. DOI 10.1002/adpr.202000098
Puc, Uros, Tobias Bach, Peter Günter, Marko Zgonik, and Mojca Jazbinsek. 2021. “Ultra‐Broadband and High‐Dynamic‐Range THz Time‐Domain Spectroscopy System Based on Organic Crystal Emitter and Detector in Transmission and Reflection Geometry.” Advanced Photonics Research 2 (4): 2000098. https://doi.org/10.1002/adpr.202000098.
Puc, Uros, et al. “Ultra‐Broadband and High‐Dynamic‐Range THz Time‐Domain Spectroscopy System Based on Organic Crystal Emitter and Detector in Transmission and Reflection Geometry.” Advanced Photonics Research, vol. 2, no. 4, 2021, p. 2000098, https://doi.org/10.1002/adpr.202000098.


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