Physics-based 0D-U-I-SoC cell performance model for aqueous organic redox flow batteries

Mourouga, Gaël; Schärer, Roman P.; Yang, Xian; Janoschka, Tobias; Schmidt, Thomas J.; Schumacher, Jürgen O.

doi:10.1016/j.electacta.2022.140185

Please use this identifier to cite or link to this item: https://doi.org/10.21256/zhaw-24719

Full metadata record

DC Field	Value	Language
dc.contributor.author	Mourouga, Gaël	-
dc.contributor.author	Schärer, Roman P.	-
dc.contributor.author	Yang, Xian	-
dc.contributor.author	Janoschka, Tobias	-
dc.contributor.author	Schmidt, Thomas J.	-
dc.contributor.author	Schumacher, Jürgen O.	-
dc.date.accessioned	2022-03-31T08:52:18Z	-
dc.date.available	2022-03-31T08:52:18Z	-
dc.date.issued	2022	-
dc.identifier.issn	0013-4686	de_CH
dc.identifier.issn	1873-3859	de_CH
dc.identifier.uri	https://digitalcollection.zhaw.ch/handle/11475/24719	-
dc.description.abstract	Aqueous organic redox-flow batteries are an emerging technological solution in the field of grid-scale energy storage, owing to their long lifetime, safety, chemical flexibility, potential for low cost and environmental friendliness. In this work we present a physics-based dimensionality reduced model for the performance prediction of aqueous organic redox flow batteries. The model allows for fast evaluations of the cell voltage and power density, which are expressed explicitly in terms of the electric current density and state of charge. The model takes into consideration important phenomena, such as the activation and concentration overpotentials in the electrodes as well as the non-negligible electro-osmotic drag of water through the membrane. A sensitivity analysis of the model indicates the influence of various model parameters at different current densities on the predicted cell voltage. In this work we found the formal potentials and ohmic cell resistance to be the most critical parameters for performance prediction. Experimental parameterization and validation on cycling and polarization experiments revealed good agreement with the experiments within a predicted range of validity due to the different simplifying assumptions.	de_CH
dc.language.iso	en	de_CH
dc.publisher	Elsevier	de_CH
dc.relation.ispartof	Electrochimica Acta	de_CH
dc.rights	http://creativecommons.org/licenses/by/4.0/	de_CH
dc.subject	AORFB	de_CH
dc.subject	Open-source software	de_CH
dc.subject	Sensitivity analysis	de_CH
dc.subject	All-organic chemical system	de_CH
dc.subject	Performance prediction	de_CH
dc.subject.ddc	621.3: Elektro-, Kommunikations-, Steuerungs- und Regelungstechnik	de_CH
dc.title	Physics-based 0D-U-I-SoC cell performance model for aqueous organic redox flow batteries	de_CH
dc.type	Beitrag in wissenschaftlicher Zeitschrift	de_CH
dcterms.type	Text	de_CH
zhaw.departement	School of Engineering	de_CH
zhaw.organisationalunit	Institute of Computational Physics (ICP)	de_CH
dc.identifier.doi	10.1016/j.electacta.2022.140185	de_CH
dc.identifier.doi	10.21256/zhaw-24719	-
zhaw.funding.eu	info:eu-repo/grantAgreement/EC/H2020/875489//Modelling for the search for new active materials for redox flow batteries/SONAR	de_CH
zhaw.issue	140185	de_CH
zhaw.originated.zhaw	Yes	de_CH
zhaw.publication.status	publishedVersion	de_CH
zhaw.volume	415	de_CH
zhaw.publication.review	Peer review (Publikation)	de_CH
zhaw.webfeed	Renewable Fuels	de_CH
zhaw.funding.zhaw	Modellierung für die Suche nach neuen aktiven Materialien für Redox-Flow-Batterien	de_CH
zhaw.author.additional	No	de_CH
zhaw.display.portrait	Yes	de_CH
Appears in collections:	Publikationen School of Engineering

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Mourouga, G., Schärer, R. P., Yang, X., Janoschka, T., Schmidt, T. J., & Schumacher, J. O. (2022). Physics-based 0D-U-I-SoC cell performance model for aqueous organic redox flow batteries. Electrochimica Acta, 415(140185). https://doi.org/10.1016/j.electacta.2022.140185

Mourouga, G. et al. (2022) ‘Physics-based 0D-U-I-SoC cell performance model for aqueous organic redox flow batteries’, Electrochimica Acta, 415(140185). Available at: https://doi.org/10.1016/j.electacta.2022.140185.

G. Mourouga, R. P. Schärer, X. Yang, T. Janoschka, T. J. Schmidt, and J. O. Schumacher, “Physics-based 0D-U-I-SoC cell performance model for aqueous organic redox flow batteries,” Electrochimica Acta, vol. 415, no. 140185, 2022, doi: 10.1016/j.electacta.2022.140185.

MOUROUGA, Gaël, Roman P. SCHÄRER, Xian YANG, Tobias JANOSCHKA, Thomas J. SCHMIDT und Jürgen O. SCHUMACHER, 2022. Physics-based 0D-U-I-SoC cell performance model for aqueous organic redox flow batteries. Electrochimica Acta. 2022. Bd. 415, Nr. 140185. DOI 10.1016/j.electacta.2022.140185

Mourouga, Gaël, Roman P. Schärer, Xian Yang, Tobias Janoschka, Thomas J. Schmidt, and Jürgen O. Schumacher. 2022. “Physics-Based 0D-U-I-SoC Cell Performance Model for Aqueous Organic Redox Flow Batteries.” Electrochimica Acta 415 (140185). https://doi.org/10.1016/j.electacta.2022.140185.

Mourouga, Gaël, et al. “Physics-Based 0D-U-I-SoC Cell Performance Model for Aqueous Organic Redox Flow Batteries.” Electrochimica Acta, vol. 415, no. 140185, 2022, https://doi.org/10.1016/j.electacta.2022.140185.