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dc.contributor.authorTan, Liguo-
dc.contributor.authorZhou, Junjie-
dc.contributor.authorZhao, Xing-
dc.contributor.authorWang, Siyang-
dc.contributor.authorLi, Minghao-
dc.contributor.authorJiang, Chaofan-
dc.contributor.authorLi, Hang-
dc.contributor.authorZhang, Yu-
dc.contributor.authorYe, Yiran-
dc.contributor.authorTress, Wolfgang-
dc.contributor.authorDing, Liming-
dc.contributor.authorGrätzel, Michael-
dc.contributor.authorYi, Chenyi-
dc.date.accessioned2024-03-01T08:13:49Z-
dc.date.available2024-03-01T08:13:49Z-
dc.date.issued2023-03-
dc.identifier.issn0935-9648de_CH
dc.identifier.issn1521-4095de_CH
dc.identifier.urihttps://digitalcollection.zhaw.ch/handle/11475/30064-
dc.description.abstractOrganic-inorganic hybrid perovskites exhibit outstanding performances in perovskite solar cells (PSCs). However, the complex solution chemistry of perovskites precursors renders it difficult to prepare large-area devices in a reproducible way, which is a prerequisite for the technology to make an impact beyond lab scale. Vacuum processing, instead, is an established technology for large-scale coating of thin films. However, with respect to the hybrid perovskites it is highly challenging due to the high vapor pressure of the organic ammonium halide. In this work, vacuum evaporation of lead iodide and solution processing of organic ammonium halide is combined to produce large-area homogeneous perovskite films with large grains in a highly reproducible way. The resulting PSCs achieve a power conversion efficiency (PCE) of 24.3% (certified 23.9%) on small area (0.10 cm2 ), 24.0% (certified 23.7%) on large area (1 cm2 ) and 20.0% for minimodule (16 cm2 ), and maintain 90% of its initial efficiency after 1000 h 1-sun operation. The vacuum evaporation prevents advert environmental effects on lead halide formation and guarantees a reproducible fabrication of high-quality large-area perovskite films, which opens a promising way for large-scale fabrication of perovskite optoelectronics.de_CH
dc.language.isoende_CH
dc.publisherWileyde_CH
dc.relation.ispartofAdvanced Materialsde_CH
dc.rightsLicence according to publishing contractde_CH
dc.subjectHigh efficiencyde_CH
dc.subjectLarge-areade_CH
dc.subjectPerovskite solar cellsde_CH
dc.subjectVacuum evaporationde_CH
dc.subject.ddc621.3: Elektro-, Kommunikations-, Steuerungs- und Regelungstechnikde_CH
dc.titleCombined vacuum evaporation and solution process for high-efficiency large-area perovskite solar cells with exceptional reproducibilityde_CH
dc.typeBeitrag in wissenschaftlicher Zeitschriftde_CH
dcterms.typeTextde_CH
zhaw.departementSchool of Engineeringde_CH
zhaw.organisationalunitInstitute of Computational Physics (ICP)de_CH
dc.identifier.doi10.1002/adma.202205027de_CH
dc.identifier.pmid36681866de_CH
zhaw.funding.euNode_CH
zhaw.issue13de_CH
zhaw.originated.zhawYesde_CH
zhaw.pages.starte2205027de_CH
zhaw.publication.statuspublishedVersionde_CH
zhaw.volume35de_CH
zhaw.publication.reviewPeer review (Publikation)de_CH
zhaw.webfeedPhotovoltaikde_CH
zhaw.author.additionalNode_CH
zhaw.display.portraitYesde_CH
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Tan, L., Zhou, J., Zhao, X., Wang, S., Li, M., Jiang, C., Li, H., Zhang, Y., Ye, Y., Tress, W., Ding, L., Grätzel, M., & Yi, C. (2023). Combined vacuum evaporation and solution process for high-efficiency large-area perovskite solar cells with exceptional reproducibility. Advanced Materials, 35(13), e2205027. https://doi.org/10.1002/adma.202205027
Tan, L. et al. (2023) ‘Combined vacuum evaporation and solution process for high-efficiency large-area perovskite solar cells with exceptional reproducibility’, Advanced Materials, 35(13), p. e2205027. Available at: https://doi.org/10.1002/adma.202205027.
L. Tan et al., “Combined vacuum evaporation and solution process for high-efficiency large-area perovskite solar cells with exceptional reproducibility,” Advanced Materials, vol. 35, no. 13, p. e2205027, Mar. 2023, doi: 10.1002/adma.202205027.
TAN, Liguo, Junjie ZHOU, Xing ZHAO, Siyang WANG, Minghao LI, Chaofan JIANG, Hang LI, Yu ZHANG, Yiran YE, Wolfgang TRESS, Liming DING, Michael GRÄTZEL und Chenyi YI, 2023. Combined vacuum evaporation and solution process for high-efficiency large-area perovskite solar cells with exceptional reproducibility. Advanced Materials. März 2023. Bd. 35, Nr. 13, S. e2205027. DOI 10.1002/adma.202205027
Tan, Liguo, Junjie Zhou, Xing Zhao, Siyang Wang, Minghao Li, Chaofan Jiang, Hang Li, et al. 2023. “Combined Vacuum Evaporation and Solution Process for High-Efficiency Large-Area Perovskite Solar Cells with Exceptional Reproducibility.” Advanced Materials 35 (13): e2205027. https://doi.org/10.1002/adma.202205027.
Tan, Liguo, et al. “Combined Vacuum Evaporation and Solution Process for High-Efficiency Large-Area Perovskite Solar Cells with Exceptional Reproducibility.” Advanced Materials, vol. 35, no. 13, Mar. 2023, p. e2205027, https://doi.org/10.1002/adma.202205027.


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